Emitters for fast-spectrum self-powered neutron detector

Patent metadata

Field	Value
Publication number	US-12099153-B2
Application number	US-202117510044-A
Country	US
Kind code	B2
Filing date	Oct 25, 2021
Priority date	Nov 13, 2020
Publication date	Sep 24, 2024
Grant date	Sep 24, 2024

Abstract

A detector for generating an electrical current that is proportional to a flux of neutrons includes a neutron sensitive emitter, a conductive collector, an insulator between the neutron-sensitive emitter and the collector, an electrical connection to the neutron sensitive emitter, and an electrical connection to the conductive collector. The neutron sensitive emitter includes an emitter material with no more than 2 stable isotopes, and which upon impact by a neutron having an energy of from 100 keV to 1000 keV will generate electrons in proportion to the flux of neutrons in less than 10 minutes, and any generated electrons not generated in less than 10 minutes will be generated in no less than 30 days. A method of detecting neutrons generated by a nuclear reactor is also disclosed.

First claim

We claim:

1. A self-powered fast neutron detector for generating an electrical current that is proportional to a flux of neutrons, comprising:
a neutron sensitive emitter;
a conductive collector;
an insulator between the neutron-sensitive emitter and the collector;
an electrical connection to the neutron sensitive emitter; and
an electrical connection to the conductive collector;
wherein the neutron sensitive emitter comprises a Ta alloy of at least one selected from the group consisting of ASTAR-811C and T-111 and comprises an emitter material with no more than 2 stable isotopes, and which upon impact by a neutron having an energy of from 100 keV to 1000 keV will generate electrons in proportion to the flux of neutrons in less than 10 minutes, and any additional generated electrons not generated in less than 10 minutes will be generated in no less than 30 days; and
wherein the detector provides a signal to noise ratio of greater than 1.5 for neutrons having an energy of between 100 keV and 1000 keV, wherein the signal is associated with electrons generated in less than 10 minutes and the noise is associated with electrons generated in more than 10 minutes.

2. The detector of claim 1 , wherein the neutron-sensitive emitter comprises at least one emitter material selected from the group consisting of 181 Ta, 159 Tb, and 169 Tm.

3. The detector of claim 1 , wherein the neutron-sensitive emitter comprises at least one emitter material selected from the group consisting of Lu and Ir.

4. The detector of claim 3 , wherein the Lu comprises in the neutron-sensitive emitter is at least one emitter material selected from the group consisting of 175 Lu and 176 Lu.

5. The detector of claim 3 , wherein the Ir comprises at least one emitter material selected from the group consisting of 191 Ir and 193 Ir.

6. The detector of claim 1 , wherein the insulator comprises at least one selected from the group consisting of MgO, Al 2 O 3 , and vacuum.

7. The detector of claim 1 , wherein the collector is a sheath with an open interior, and the emitter and the insulator are positioned within the interior.

8. The detector of claim 7 , wherein the emitter material is provided on a conductive support mounted within the open interior of the collector sheath, and the insulator is positioned between the emitter material and the collector sheath.

9. The detector of claim 1 , wherein the collector comprises stainless steel.

10. The detector of claim 1 , wherein the collector comprises Inconel.

11. The detector of claim 1 , further comprising a current meter for measuring the electrical current generated by the flux of neutrons striking the emitter.

12. The detector of claim 11 , further comprising a processor for relating the current measured by the current meter to the neutron flux.

13. A method of detecting neutrons generated by a nuclear reactor, comprising the steps of:
providing a self-powered fast neutron detector comprising a neutron sensitive emitter; a conductive collector; an insulator between the neutron-sensitive emitter and the collector; and an electrical connection to the neutron sensitive emitter;
providing an electrical connection to the conductive collector; wherein the neutron sensitive emitter comprises a Ta alloy of an emitter material comprising at least one selected from the group consisting of 159 Tb and 169 Tm and at least one selected from the group consisting of ASTAR-811C and T-111, the emitter material having no more than 2 stable isotopes, and which upon impact by a neutron having an energy of from 100 keV to 1000 keV will generate electrons in proportion to the flux of neutrons in less than 10 minutes or more than 30 days;
exposing the neutron detector to neutrons having an energy of from 100 keV to 1000 keV, wherein electrons will be generated by the emitter material in proportion to the flux in less than 10 minutes, and any additional generated electrons not generated in less than 10 minutes will be generated in no less than 30 days;
the detector generating a signal to noise ratio of greater than 1.5 for neutrons having an energy of between 100 keV and 1000 keV; wherein the signal is associated with electrons generated in less than 10 minutes, and the noise is associated with electrons generated in more than 10 minutes;
using a current meter to measure the electrical current generated by the flux of neutrons striking the emitter; and,
using a processor to relate the current measured by the current meter to the neutron flux.

14. The method of claim 13 , wherein electrons are generated in less than 5 minutes.

15. The method of claim 14 , wherein any electron not generated in less than 5 minutes will be generated in no less than 72 days.

16. The method of claim 13 , wherein the nuclear reactor is configured and operated as a fast-spectrum nuclear reactor.

Assignees

• Ut Battelle Llc

Inventors

• Goetz Kathleen C
• Cetiner Mustafa S

Classifications

• G21C17/108 Primary

  Measuring reactor flux · CPC title

• G21C17/102

  the sensitive element being part of a fuel element or a fuel assembly (structural combination with a thermoelectric element for direct production of electrical energy G21C3/40) · CPC title

• Y02E30/30

  Nuclear fission reactors · CPC title

• G01T3/006 Primary

  using self-powered detectors (for neutrons as well as for Y- or X-rays), e.g. using Compton-effect (Compton diodes) or photo-emission or a (n,B) nuclear reaction (radioisotopic generators G21H1/00, e.g. G21H1/02, G21H1/04; photo-tubes H01J40/00; thermionic generators H01J45/00) · CPC title