Mullite-containing sintered body, method for manufacturing the same, and composite substrate

Patent metadata

Field	Value
Publication number	US-9981876-B2
Application number	US-201715454180-A
Country	US
Kind code	B2
Filing date	Mar 9, 2017
Priority date	Mar 23, 2016
Publication date	May 29, 2018
Grant date	May 29, 2018

Abstract

A mullite-containing sintered body according to the present invention contains mullite and at least one selected from the group consisting of silicon nitride, silicon oxynitride, and sialon. It is preferable that the mullite-containing sintered body have a thermal expansion coefficient of less than 4.3 ppm/° C. at 40° C. to 400° C., an open porosity of 0.5% or less, and an average grain size of 1.5 μm or less.

First claim

What is claimed is:

1. A mullite-containing sintered body comprising mullite and at least one selected from the group consisting of silicon nitride, silicon oxynitride, and sialon,
wherein the thermal expansion coefficient is less than 4.3 ppm/° C. at 40° C. to 400° C.,
the open porosity is 0.5% or less, and
the average grain size is 1.5 μm or less.

2. The mullite-containing sintered body according to claim 1 ,
wherein the number of pores that have a maximum length of 1 μm or more present in an area of 100 μm×100 μm of a polished surface is 10 or less.

3. The mullite-containing sintered body according to claim 1 ,
wherein the Young's modulus is 240 GPa or more.

4. The mullite-containing sintered body according to claim 1 ,
wherein the four-point bending strength is 320 MPa or more.

5. The mullite-containing sintered body according to claim 1 ,
wherein the center line average roughness Ra of the polished surface is 1.5 nm or less.

6. A method for manufacturing a mullite-containing sintered body according to claim 1 comprising:
(a) producing a mixed raw material powder by mixing 50 to 90 percent by volume of mullite powder having an average particle diameter of 1.5 μm or less and 10 to 50 percent by volume of silicon nitride powder having an average particle diameter of 1 μm or less such that the total is 100 percent by volume, and
(b) producing the mullite-containing sintered body by forming the mixed raw material powder into a compact having a predetermined shape and subjecting the compact to hot press firing at a pressing pressure of 20 to 300 kgf/cm 2 and a firing temperature of 1,525° C. to 1,700° C.

7. A composite substrate in which a functional substrate is bonded to a support substrate,
wherein the support substrate is the mullite-containing sintered body according to claim 1 .

Assignees

• Ngk Insulators Ltd

Inventors

• Isoda Yoshinori
• Suzuki Yoshio
• Inoue Katsuhiro
• Katsuda Yuji

Classifications

• C04B2237/341

  Silica or silicates · CPC title

• B32B2250/02

  2 layers · CPC title

• C04B2235/6567

  Treatment time · CPC title

• C04B35/185 Primary

  Mullite {3Al2O3-2SiO2} · CPC title

• C04B2235/80

  Phases present in the sintered or melt-cast ceramic products other than the main phase · CPC title