Interconnector material, intercellular separation structure, and solid electrolyte fuel cell

Patent metadata

Field	Value
Publication number	US-9941524-B2
Application number	US-201414456658-A
Country	US
Kind code	B2
Filing date	Aug 11, 2014
Priority date	Jul 14, 2008
Publication date	Apr 10, 2018
Grant date	Apr 10, 2018

Abstract

Provided is an interconnector material which is chemically stable in both oxidation atmospheres and reduction atmospheres, has a high electron conductivity (electric conductivity), a low ionic conductivity, does not contain Cr, and enables a reduction in sintering temperature. The interconnector material is arranged between a plurality of cells each composed of an anode layer, a solid electrolyte layer, and a cathode layer stacked sequentially, and electrically connects the plurality of cells to each other in series in a solid electrolyte fuel cell. The interconnector is formed of a ceramic composition represented by the composition formula La(Fe 1-x Al x )O 3 in which 0<x<0.5.

First claim

The invention claimed is:

1. A cell structure comprising:
a plurality of cells which each comprise
an anode layer,
a solid electrolyte layer,
a cathode layer stacked sequentially; and

an intercellular separation structure disposed between cells of the plurality of cells,
the intercellular separation structure comprising an electrical insulator disposed to separate an anode gas and a cathode gas which are supplied to each of the plurality of cells and an electrical conductor in the electrical insulator electrically connecting the plurality of cells to each other, and
the electrical conductor comprising a first conductive body electrically connected to the anode layer, a second conductive body electrically connected to the cathode layer, and an interconnector of dense material through which a gas does not a pass disposed to connect the first conductive body and second conductive body.

2. The solid electrolytic fuel cell structure according to claim 1 wherein
the anode layer comprises a fuel electrode and the cathode layer comprises an air electrode,
the first conductive body contacts the anode layer through the fuel electrode, and
the second conductive body contacts the cathode layer through the air electrode.

3. The solid electrolyte fuel cell according to claim 2 , wherein the anode layer comprises nickel.

4. The solid electrolytic fuel cell structure according to claim 3 wherein the interconnector comprises a ceramic component electrical conductor having a compositional formula of La(Fe 1-x Al x )O 3 in which 0<x<0.5.

5. The solid electrolytic fuel cell structure according to claim 2 wherein the interconnector comprises a ceramic component electrical conductor having a compositional formula of La(Fe 1-x Al x )O 3 in which 0<x<0.5.

6. The solid electrolytic fuel cell structure according to claim 5 , wherein 0.1≤x≤0.3.

7. The solid electrolytic fuel cell structure according to claim 1 wherein the interconnector comprises a ceramic component electrical conductor having a compositional formula of La(Fe 1-x Al x )O 3 in which 0<x<0.5.

8. The solid electrolytic fuel cell structure according to claim 5 , wherein 0.1≤x≤0.3.

9. The solid electrolyte fuel cell according to claim 8 , wherein the anode layer comprises nickel.

10. The solid electrolyte fuel cell according to claim 1 , wherein the anode layer comprises nickel.

11. The solid electrolyte fuel cell according to claim 1 , further comprising:
a first current collecting layer disposed between the anode layer and the first conductive body; and
a second current collecting layer disposed between the cathode layer and the second conductive body.

Assignees

• Murata Manufacturing Co

Inventors

• Takata Kazuhide
• Iha Michiaki

Classifications

• C04B2237/346

  Titania or titanates · CPC title

• C04B37/006

  consisting of metals or metal salts · CPC title

• C04B38/068

  Carbonaceous materials, e.g. coal, carbon, graphite, hydrocarbons · CPC title

• C04B2237/62

  Forming laminates or joined articles comprising holes, channels or other types of openings · CPC title

• C04B2237/34

  Oxidic · CPC title