Methods for gas leak detection and localization in populated areas using isotope ratio measurements

Patent metadata

Field	Value
Publication number	US-9739758-B2
Application number	US-201414493853-A
Country	US
Kind code	B2
Filing date	Sep 23, 2014
Priority date	Oct 20, 2011
Publication date	Aug 22, 2017
Grant date	Aug 22, 2017

Abstract

Improved gas leak detection from moving platforms is provided. Automatic horizontal spatial scale analysis can be performed in order to distinguish a leak from background levels of the measured gas. Source identification can be provided by using isotopic ratios and/or chemical tracers to distinguish gas leaks from other sources of the measured gas. Multi-point measurements combined with spatial analysis of the multi-point measurement results can provide leak source distance estimates. Qualitative source identification is provided. These methods can be practiced individually or in any combination.

First claim

The invention claimed is:

1. A method of gas leak detection and localization, the method comprising:
performing one or more primary gas concentration measurements from a moving platform that proceeds along at least one platform track disposed in proximity to one or more potential gas leak locations of utility infrastructure, wherein the moving platform is a terrestrial moving platform;
performing one or more secondary isotope ratio measurements from the moving platform as it proceeds along the at least one platform track, wherein the secondary isotope ratio measurements are analyzed on-board the moving platform;
automatically determining whether or not a gas leak is present at the potential gas leak locations based on the primary gas concentration measurements and the secondary isotope ratio measurements, wherein the secondary isotope ratio measurements provide qualitative source identification for detected leaks; and
providing a leak indication at the potential gas leak locations to an end user;
wherein the primary gas concentration measurements are local measurements of gas concentration at the moving platform;
wherein the one or more secondary isotope ratio measurements are measurements of relative abundance of isotopes within a chemical species detected by the primary gas concentration measurements;
wherein isotopes are atoms having nuclei with an equal number of protons and an unequal number of neutrons;
wherein the qualitative source identification comprises estimation based on likelihoods of two or more possible source types
wherein the qualitative source identification comprises computing posterior probabilities according to Bayes' Theorem and attributing a source type to results where the posterior probability exceeds a predetermined threshold.

2. The method of claim 1 , further comprising providing a display showing a map with the qualitative source identification for each detected leak.

3. The method of claim 1 , wherein the qualitative source identification comprises computing a linear fit of isotope ratio vs. inverse concentration, and computing a y-intercept of the linear fit.

4. The method of claim 1 , wherein multiple measurement results are used to compute the posterior probabilities.

5. The method of claim 1 , wherein the likelihoods are dependent on a location of the primary gas concentration measurements.

6. The method of claim 1 , wherein the likelihoods are dependent on a priori knowledge of isotopic compositions of one or more of the possible source types.

7. The method of claim 3 , wherein the qualitative source identification further comprises providing a qualitative result based on the linear fit and wherein the qualitative result comprises a result selected from the group consisting of: natural gas and not natural gas.

8. The method of claim 3 , wherein the qualitative source identification further comprises computing an estimated uncertainty of the y-intercept.

9. The method of claim 8 , wherein the qualitative source identification further comprises providing a qualitative result based on the linear fit and wherein the qualitative result comprises a result selected from the group consisting of: natural gas, not natural gas, and unknown.

10. The method of claim 9 , wherein the unknown result is provided if the uncertainty of the y-intercept exceeds a predetermined value.

11. The method of claim 9 , wherein the unknown result is provided if the estimated uncertainty of the y-intercept provides a range of y-intercepts that overlaps with a boundary between y-intercept ranges having different predetermined assigned qualitative results.

Assignees

• Picarro Inc

Inventors

• Rella Chris W
• Crosson Eric R
• Woelk Michael R
• Tan Sze Meng
• He Yonggang
• Steele David

Classifications

• G01N21/39

  using tunable lasers · CPC title

• G01M3/20

  using special tracer materials, e.g. dye, fluorescent material, radioactive material · CPC title

• G01M3/38

  by using light (G01M3/02 takes precedence) · CPC title

• G01N21/01

  Arrangements or apparatus for facilitating the optical investigation · CPC title

• G01N33/0009 Primary

  General constructional details of gas analysers, e.g. portable test equipment (devices for withdrawing samples in the gaseous state G01N1/22) · CPC title