Rare-earth bond magnet manufacturing method

Patent metadata

Field	Value
Publication number	US-9666361-B2
Application number	US-201213985152-A
Country	US
Kind code	B2
Filing date	Feb 27, 2012
Priority date	Mar 2, 2011
Publication date	May 30, 2017
Grant date	May 30, 2017

Abstract

A method for producing a bonded rare-earth magnet according to an embodiment of the present invention includes the steps of: providing a rapidly solidified rare-earth magnet alloy powder; providing a solution in which a resin that is in solid phase at an ordinary temperature is dissolved in an organic solvent; mulling the rapidly solidified rare-earth magnet alloy powder and the solution together and vaporizing the organic solvent, thereby making a bonded rare-earth magnet compound in which magnet powder particles that form the rapidly solidified rare-earth magnet alloy powder are coated with the resin; making a compressed compact by compressing the bonded rare-earth magnet compound under a pressure of 1000 MPa to 2500 MPa; and thermally treating the compressed compact. If the rapidly solidified rare-earth magnet alloy powder to be mulled is 100 mass %, the solution includes 0.4 mass % to 1.0 mass % of the resin and 1.2 mass % to 20 mass % of the organic solvent.

First claim

The invention claimed is:

1. A method for producing a bonded rare-earth magnet, the method comprising the steps of:
providing a rapidly solidified rare-earth magnet alloy powder consisting of particles each having a flat shape, wherein a ratio of a minor axis size of the flat shape to a major axis size of the flat shape is 0.3 or less and wherein a 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder is within a range of 75 μm to 105 μm;
providing a solution in which a resin that is in solid phase at room temperature is dissolved in an organic solvent;
mulling the rapidly solidified rare-earth magnet alloy powder and the solution together and vaporizing the organic solvent, thereby making a bonded rare-earth magnet compound in which magnet powder particles that form the rapidly solidified rare-earth magnet alloy powder are coated with the resin, wherein each particle contained in the bonded rare-earth magnet compound has the flat shape, wherein the ratio of the minor axis size of the flat shape to the major axis size of the flat shape is 0.3 or less, and wherein the 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder coated with the resin is within the range of 75 μm to 105 μm;
making a compressed compact by compressing the bonded rare-earth magnet compound under a pressure of 1000 MPa to 2500 MPa; and
thermally treating the compressed compact to form a bonded rare-earth magnet having a density of approximately 6.4 to 6.6 g/cm 3 , wherein
if the rapidly solidified rare-earth magnet alloy powder to be mulled is 100 mass %, the solution includes 0.4 mass % to 1.0 mass % of the resin and 1.2 mass % to 20 mass % of the organic solvent, the resin including a curing agent,
in the bonded rare-earth magnet compound, the resin including the curing agent coats the magnet powder particles at a coverage of 90% or more,
the resin including the curing agent that coats the magnet powder particles has a thickness of 0.1 μm to 1 μm, and
a gap between adjacent ones of the magnet powder particles each having the flat shape is 2 μm or less as measured in a cross section parallel to a compressing direction.

2. The method of claim 1 , comprising the steps of:
subjecting the compressed compact to a barrel process after the step of thermally treating;
dipping the compressed compact that has been subjected to the barrel process in a resin solution that has been diluted with an organic solvent and that includes 2 to 13 mass % of thermosetting resin component; and
removing the compressed compact from the resin solution and drying the compressed compact.

3. The method of claim 1 , wherein the compressed compact is made by compressing the bonded rare-earth magnet compound under a pressure of 1960 MPa to 2500 MPa.

4. A method for producing a bonded rare-earth magnet, the method comprising the steps of:
providing a rapidly solidified rare-earth magnet alloy powder consisting of particles each having a flat shape, wherein a ratio of minor axis size of the flat shape to a major axis size of the flat shape is 0.3 or less, and wherein a 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder is within a range of 75 μm to 105 μm;
providing a solution in which a resin that is in solid phase at room temperature is dissolved in an organic solvent;
mulling the rapidly solidified rare-earth magnet alloy powder and the solution together and vaporizing the organic solvent, thereby making a bonded rare-earth magnet compound in which magnet powder particles that form the rapidly solidified rare-earth magnet alloy powder are coated with the resin, wherein each particle contained in the bonded rare-earth magnet compound has the flat shape, wherein the ratio of the minor axis size of the flat shape to the major axis size of the flat shape is 0.3 or less, and wherein the 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder coated with the resin is within the range of 75 μm to 105 μm;
making a compressed compact by compressing the bonded rare-earth magnet compound under a pressure of 1000 MPa to 2500 MPa; and
thermally treating the compressed compact to form a bonded rare-earth magnet having a density of approximately 6.4 to 6.6 g/cm 3 , the bonded magnet having a mechanical strength of 30 MPa or more, wherein
if the rapidly solidified rare-earth magnet alloy powder to be mulled is 100 mass %, the solution includes 0.4 mass % to 1.0 mass % of the resin and 1.2 mass % to 20 mass % of the organic solvent, the resin including a curing agent,
in the bonded rare-earth magnet compound, the resin including the curing agent coats the magnet powder particles at a coverage of 90% or more,
the resin including the curing agent that coats the magnet powder particles has a thickness of 0.1 μm to 1 μm, and
a gap between adjacent ones of the magnet alloy powder particles each having the flat shape is 2 μm or less as measured in a cross section parallel to a compressing direction.

5. The method of claim 4 , wherein the compressed compact is made by compressing the bonded rare-earth magnet compound under a pressure of 1960 MPa to 2500 MPa.

6. A method for producing a bonded rare-earth magnet, the method comprising the steps of:
providing a rapidly solidified rare-earth magnet alloy powder consisting of particles each having a flat shape, wherein a ratio of minor axis size of the flat shape to a major axis size of the flat shape is 0.3 or less, and wherein a 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder is within a range of 75 μm to 105 μm;
providing a solution in which a resin that is in solid phase at room temperature is dissolved in an organic solvent;
mulling the rapidly solidified rare-earth magnet alloy powder and the solution together and vaporizing the organic solvent, thereby making a bonded rare-earth magnet compound in which magnet powder particles that form the rapidly solidified rare-earth magnet alloy powder are coated with the resin, wherein each particle contained in the bonded rare-earth magnet compound has the flat shape, wherein the ratio of the minor axis size of the flat shape to the major axis size of the flat shape is 0.3 or less, and wherein the 50 mass % particle size of the rapidly solidified rare-earth magnet alloy powder coated with the resin is within the range of 75 μm to 105 μm;
making a compressed compact by compressing the bonded rare-earth magnet compound under a pressure of 1000 MPa to 2500 MPa; and
thermally treating the compressed compact to form a bonded rare-earth magnet having a density of approximately 6.4 to 6.6 g/cm 3 , the bonded magnet having an electrical resistance of 1600 μΩ·m or more, wherein
if the rapidly solidified rare-earth magnet alloy powder to be mulled is 100 mass %, the solution includes 0.4 mass % to 1.0 mass % of the resin and 1.2 mass % to 20 mass % of the organic solvent, the resin including a curing agent,
in the bonded rare-earth magnet compound, the resin including the curing agent coats the magnet powder particles at a coverage of 90% or more,
the resin including the curing agent that coats the magnet powder particles has a thickness of 0.1 μm to 1 μm, and
a gap between adjacent ones of the magnet alloy particles each having the flat shape is 2 μm or less as measured in a cross section parallel to a compressing direction.

7. The method of claim 6 , wherein the bonded magnet has a mechanical strength of 30 MPa or more.

8. The method of claim 6 , wherein the compressed compact is made by compressing the bonded rare-earth magnet compound under a pressure of 1960 MPa to 2500 MPa.

Assignees

• Takayama Kazuhiro
• Miyoshi Toshio
• Hitachi Metals Ltd

Inventors

• Takayama Kazuhiro
• Miyoshi Toshio

Classifications

• B22F1/102

  Metallic powder coated with organic material · CPC title

• B22F3/02 Primary

  Compacting only · CPC title

• B23K35/3613

  Polymers, e.g. resins · CPC title

• H01F41/005

  Impregnating or encapsulating (insulating of windings H01F41/12) · CPC title

• C22C1/04

  by powder metallurgy (C22C1/08 takes precedence) · CPC title