Fabrication method of burnable absorber nuclear fuel pellets and burnable absorber nuclear fuel pellets fabricated by the same

Patent metadata

Field	Value
Publication number	US-9653188-B2
Application number	US-201313747685-A
Country	US
Kind code	B2
Filing date	Jan 23, 2013
Priority date	Feb 28, 2012
Publication date	May 16, 2017
Grant date	May 16, 2017

Abstract

A fabrication method of burnable absorber nuclear fuel pellets and burnable absorber nuclear fuel pellets fabricated by the same are provided, in which the fabrication method includes adding boron compound and manganese compound to one or more type of nuclear fuel powders selected from the group consisting of uranium dioxide (UO 2 ), plutonium dioxide (PuO 2 ) and thorium dioxide (ThO 2 ) and mixing the same (step 1), compacting the mixed powder of step 1 into compacts (step 2), and sintering the compacts of step 2 under hydrogen atmosphere (step 3). According to the fabrication method, sintering can be performed under hydrogen atmosphere at a temperature lower than the hydrogen atmosphere sintering that is conventionally applied in the nuclear fuel sintered pellet mass production, by adding sintering additives such as manganese oxide or the like.

First claim

What is claimed is:

1. A fabrication method of burnable absorber nuclear fuel pellets, comprising:
adding a boron compound, which is one or more of compounds selected from the group consisting of boron carbide (B 4 C), titanium diboride (TiB 2 ), zirconium diboride (ZrB 2 ) and boron nitride (BN) and a manganese compound to one or more of nuclear fuel powders selected from the group consisting of uranium dioxide (UO 2 ), plutonium dioxide (PuO 2 ) and thorium dioxide (ThO 2 ) and mixing the same (step 1);
compacting the mixed powder of step 1 into compacts (step 2); and
sintering the compacts of step 2 under a hydrogen atmosphere (step 3) performed at a temperature range of between about 1000° C. and about 1500° C., wherein, upon sintering, the nuclear fuel pellets have a density of 90% TD (theoretical density) or above, wherein the boron compound of step 1 is added in an amount of 0.01 to 5 wt. % per nuclear fuel powder, and the manganese compound of step 1 is added in an amount of 0.01 to 1 wt. % per nuclear fuel powder, and mixed therein,
wherein the boron compound and the manganese compound are uniformly dispersed in the compacts of step 2.

2. The fabrication method of claim 1 , wherein the boron compound of step 1 is boron nitride (BN).

3. The fabrication method of claim 1 , wherein the manganese compound of step 1 is one or more of compounds selected from the group consisting of manganese oxide (MnO), manganese dioxide (MnO 2 ), manganese sulfide, manganese fluoride, and manganese chloride.

4. The fabrication method of claim 1 , wherein the manganese compound of step 1 is manganese oxide (MnO).

5. The fabrication method of claim 1 , wherein the compacts of step 2 are formed under pressure of 1 to 5 ton/cm 2 .

6. The fabrication method of claim 1 , wherein the sintering of step 3 is performed at a temperature range of 1000 to 1200 degree C.

7. The fabrication method of claim 1 , wherein the hydrogen atmosphere further comprises one or more of gases selected from the group consisting of argon, nitrogen, carbon dioxide and water vapor.

Assignees

• Korea Atomic Energy Res

Inventors

• Rhee Young Woo
• Kim Dong-Joo
• Kim Jong-Hun
• Yang Jae-Jo
• Kim Keon-Sik
• Koo Yang-Hyun

Classifications

• G21C3/623

  Oxide fuels · CPC title

• G21C3/326 Primary

  comprising fuel elements of different composition; comprising, in addition to the fuel elements, other pin-, rod-, or tube-shaped elements, e.g. control rods, grid support rods, fertile rods, poison rods or dummy rods · CPC title

• G21C21/02

  Manufacture of fuel elements or breeder elements contained in non-active casings · CPC title

• G21C3/20 Primary

  with coating on fuel or on inside of casing; with non-active interlayer between casing and active material {with multiple casings or multiple active layers} · CPC title

• G21C3/42 Primary

  Selection of substances for use as reactor fuel · CPC title