Direct sealing of glass microstructures

Patent metadata

Field	Value
Publication number	US-9527724-B2
Application number	US-201113989897-A
Country	US
Kind code	B2
Filing date	Nov 28, 2011
Priority date	Nov 30, 2010
Publication date	Dec 27, 2016
Grant date	Dec 27, 2016

Abstract

Embodiments of methods for sealing a glass microstructure assembly comprise providing one or more side retainer members on a base plate adjacent the glass microstructure assembly, the side retainer members having a height less than an uncompressed height defined by the glass microstructure assembly. The methods also comprise compressing the glass microstructure assembly via a load bearing top plate in intimate contact with the top glass layer while heating the glass microstructure assembly and the top plate to a glass sealing temperature, the glass sealing temperature being a temperature sufficient to make glass viscous, wherein the glass microstructure assembly is compressed until the load bearing top plate contacts the side retainer members, and wherein the lower surface of the top plate maintains adhesion to the upper surface of the top glass layer at the glass sealing temperature while the load bearing plate is supported by the side retainer members.

First claim

What is claimed is:

1. A method of sealing a glass microstructure assembly comprising:
providing a base plate as a support for the glass microstructure assembly;
providing the glass microstructure assembly comprising,
one or more patterned glass layers disposed over the base plate, and
a top glass layer stacked on the one or more patterned glass layers, the one or more patterned glass layers and the top glass layer comprising a glass;
wherein at least a first channel is formed between the top glass layer and the one or more patterned glass layers,

providing a load bearing top plate on an upper surface of the top glass layer such that a lower surface of the top plate intimately contacts the upper surface of the top glass layer, the top plate and the base plate being comprised of a non-glass composition;
providing one or more side retainer members on the base plate adjacent the glass microstructure assembly, the one or more side retainer members extending upwardly a vertical distance less than an uncompressed height defined by the glass microstructure assembly;
compressing the glass microstructure assembly via the load bearing top plate in intimate contact with the top glass layer while heating the glass microstructure and the top plate to a glass sealing temperature, the glass sealing temperature being a temperature sufficient to make the glass of the one or more patterned glass layers and the top glass layer viscoelastic with a viscosity of 10 6 to 10 9 poises, the load bearing top plate vertically compressing the glass until the load bearing top plate contacts and is supported by the one or more side retainer members, and the lower surface of the top plate adhering to the upper surface of the top glass layer at the glass sealing temperature while the load bearing plate is supported by the side retainer members.

2. The method of claim 1 wherein the load bearing top plate comprises a composition that does not adhere to the glass microstructure assembly at room temperature.

3. The method of claim 1 wherein the load bearing top plate has a flat lower surface, and the top glass layer has a substantially flat upper surface.

4. The method of claim 1 wherein the one or more side retainer members comprise alumina.

5. The method of claim 1 wherein the top plate comprises graphite.

6. The method of claim 5 wherein the graphite top plate is free of carbon soot or dust on the lower surface of the graphite top plate.

7. The method of claim 1 wherein the one or more patterned glass layers is stacked on a bottom glass layer comprising the glass, the bottom glass layer being contacted and supported by the base plate.

8. The method of claim 7 wherein the bottom glass layer defines a flat cross section on its upper and lower surfaces.

9. The method of claim 8 wherein the lower surface of the top glass layer is flat.

10. The method of claim 7 wherein at least a second channel is formed between the bottom glass layer and the one or more patterned glass layers.

11. The method of claim 1 wherein the heating of the glass microstructure assembly rounds one or more angles of the at least a first channel.

12. The method of claim 1 wherein the glass microstructure assembly is heated at the glass sealing temperature for from 2 to 4 hours.

13. The method of claim 12 wherein the glass microstructure assembly is heated at the glass sealing temperature for 3 hours.

14. The method of claim 1 further comprising cooling the glass microstructure assembly to form a glass microreactor.

15. A glass microreactor produced by the method of claim 14 .

16. A method of sealing a glass microstructure assembly comprising:
providing a glass microstructure assembly comprising,
one or more patterned glass layers disposed over a base plate, and
a top glass layer stacked on the one or more patterned glass layers
wherein at least one channel is formed between the top glass layer and the one or more patterned glass layers;

providing the base plate as a support for the glass microstructure assembly;
providing a load bearing top plate on an upper surface of the top glass layer such that a lower surface of the top plate intimately contacts the upper surface of the top glass layer, the top plate and the base plate being comprised of a non-glass composition;
providing one or more side retainer members on the base plate adjacent the glass microstructure assembly, the one or more side retainer members having a height less than an uncompressed height defined by the glass microstructure assembly;
compressing the glass microstructure assembly via the load bearing top plate in intimate contact with the top glass layer while heating the glass microstructure assembly to a glass sealing temperature, the glass sealing temperature being a temperature sufficient to make the glass of the one or more patterned glass layers and the top glass layer viscous with a viscosity of 10 6 to 10 9 poises, wherein the load bearing top plate vertically compresses the glass until the load bearing top plate contacts and is supported by the one or more side retainer members, and
wherein the lower surface of the top plate maintains adhesion to the upper surface of the top glass layer at the glass sealing temperature while the load bearing top plate is supported by the side retainer members, and
removing sharp angles of the at least one channel by maintaining the glass microstructure assembly at the glass sealing temperature from 2 to 4 hours, wherein the heating of the glass microstructure assembly increases surface tension in the glass microstructure assembly, and thereby smoothes the sharp angles of the at least one channel.

17. The method of claim 16 further comprising cooling the glass microstructure assembly to form a glass microreactor.

18. A glass microreactor produced by the method of claim 17 .

Assignees

• Dannoux Thierry Luc Alain
• Marques Paulo Gaspar Jorge
• Tanguy Ronan
• Corning Inc

Inventors

• Dannoux Thierry Luc Alain
• Marques Paulo Gaspar Jorge
• Tanguy Ronan

Classifications

• B81C2203/036

  Fusion bonding · CPC title

• B01L2300/0887

  Laminated structure · CPC title

• B01L3/502707 Primary

  characterised by the manufacture of the container or its components · CPC title

• C03B23/245

  Hollow glass sheets · CPC title

• B81C1/00357

  involving bonding one or several substrates on a non-temporary support, e.g. another substrate · CPC title