Reactor incorporating a heat exchanger

Patent metadata

Field	Value
Publication number	US-9394170-B2
Application number	US-201414205864-A
Country	US
Kind code	B2
Filing date	Mar 12, 2014
Priority date	Mar 12, 2013
Publication date	Jul 19, 2016
Grant date	Jul 19, 2016

Abstract

A reactor containing a heat exchanger is disclosed, which can be operated with co-current or counter-current flow. Also disclosed is a system that includes a reactor having a reformer and a vaporizer, a fuel supply, and a water supply. The reactor includes a source of combustion gas, a reformer operative to receive reformate, and a vaporizer operative to receive water. The reformer and vaporizer each include a stack assembly formed by a combination of separator shims and channel shims. The separator shims and channel shims are stacked in a regular pattern to form two sets of channels within the stack assembly. One set of channels will have vertical passageways at either end and a horizontal flowpath between them, while the other set of channels has only a horizontal flowpath.

First claim

The invention claimed is:

1. A system comprising:
a reactor that includes a combustion gas source, a reformer and a vaporizer;
wherein the reformer and the vaporizer each comprise:
a reaction channel having a flowpath, a first wall, a second wall opposite the first wall, an inlet manifold at a first end, and an outlet manifold at a second opposite end, the inlet manifold and the outlet manifold running orthogonal to the flowpath;
a combustion channel having a flowpath parallel to the flowpath of the reaction channel, the reaction channel and the combustion channel being separated by the first wall; and
a fin extending from the combustion channel into the reaction channel, the fin passing through the first wall and extending to the second wall; and

wherein combustion gas from the combustion gas source flows through the combustion channel of the reformer and through the combustion channel of the vaporizer.

2. The system of claim 1 , further including at least one adiabatic reformer connected to the reaction channel outlet manifold of the reformer.

3. The system of claim 1 , wherein the reaction channel of the reformer includes a catalyst.

4. The system of claim 3 , wherein the catalyst is rhodium on spinel.

5. The system of claim 3 , wherein the catalyst is inserted into the reaction channel as a catalyst insert.

6. The system of claim 5 , wherein the catalyst insert comprises a corrugated center piece coated on at least one side with the catalyst.

7. The system of claim 6 , wherein the corrugated center piece is sandwiched between two flat shims, and an inner surface of each flat shim is also coated with the catalyst.

8. The system of claim 1 , wherein the inlet manifolds of the reformer and the vaporizer are arranged so that fluids flowing through the reaction channels of the reformer and the vaporizer flow in a counter-current direction to combustion gas from the combustion gas source flowing through the combustion channels of the reformer and the vaporizer.

9. The system of claim 1 , further comprising a fuel-steam mixer that connects to the inlet manifold of the reformer reaction channel.

10. The system of claim 9 , further comprising a steam superheater that connects to the outlet manifold of the vaporizer reaction channel and feeds the fuel-steam mixer.

11. The system of claim 9 , further comprising a fuel supply that feeds the fuel-steam mixer.

12. The system of claim 1 , further comprising a water supply that connects to the inlet manifold of the vaporizer reaction channel.

13. The system of claim 1 , further comprising
a fuel-steam mixer;
a water supply for providing water to the vaporizer; and
a fuel supply for providing fuel to the fuel-steam mixer;
wherein the vaporizer generates steam from the water, the fuel-steam mixer forms a reformate mixture from the steam and the fuel which is sent to the reformer, and the reformer operates to generate hydrogen from the reformate mixture.

14. The system of claim 1 , further comprising a fuel cell assembly connected to the reactor for producing electricity.

15. The system of claim 14 , wherein the fuel assembly includes a proton exchange membrane fuel cell (PEMFC) or a solid oxide fuel cell (SOFC).

16. The system of claim 1 , wherein the combustion gas source is located at one end of the reactor, an exhaust port is located at an opposite end of the reactor, and the reformer combustion channel and the vaporizer combustion channel are located in series between the combustion gas source and the exhaust port.

17. The system of claim 1 , wherein the combustion gas source is located at a burner end of the device, and wherein the combustion channel includes (i) a first leg running from the burner end to an opposite end of the device and (ii) a second leg returning from the opposite end to the burner end.

18. The system of claim 17 , wherein the reaction channel and the vaporizer channel each include (i) a first leg running from the burner end to an opposite end of the device and (ii) a second leg returning from the opposite end to the burner end.

19. The system of claim 17 , wherein the reaction channel flows counter-current to the first leg of the combustion channel and the vaporizer channel flows counter-current to the second leg of the combustion channel.

20. The system of claim 1 , wherein the reformer or the vaporizer is a stack assembly formed from a regular alternating pattern of a separator shim and a channel shim.

Assignees

• Battelle Memorial Institute

Inventors

• George Ii Paul E
• Contini Vincent
• Goshe Matthew E

Classifications

• C01B2203/066

  with fuel cells · CPC title

• B01J2219/00806

  Frames · CPC title

• B01J2219/0086

  Dimensions of the flow channels · CPC title

• C01B2203/1035

  Catalyst coated on equipment surfaces, e.g. reactor walls · CPC title

• B01J2219/00835

  Comprising catalytically active material · CPC title