Manufacturing a fuel cell membrane-electrode assembly

Patent metadata

Field	Value
Publication number	US-9276281-B2
Application number	US-201113103207-A
Country	US
Kind code	B2
Filing date	May 9, 2011
Priority date	Dec 3, 2010
Publication date	Mar 1, 2016
Grant date	Mar 1, 2016

Abstract

The present invention provides an apparatus and method for manufacturing a fuel cell membrane-electrode assembly by forming a catalyst layer, which has uniform distribution, excellent porosity, and excellent bondability to a polymer electrolyte membrane, on a metal roll by an electrospray process and transferring the catalyst layer to a polymer electrolyte membrane.

First claim

What is claimed is:

1. A method for manufacturing a fuel cell membrane-electrode assembly, the method comprising:
storing a catalyst slurry in a plurality of sprays spaced from a pair of metal drums;
applying a voltage between the sprays and the metal drums;
injecting the catalyst slurry through a tip of each of the sprays toward the metal drums, wherein the catalyst slurry and voltage cause a Coulomb explosion to coat the catalyst slurry on the metal drums as a catalyst layer; and
transferring the catalyst layer to both surfaces of a polymer electrolyte membrane fed by rotation through the metal drums,
wherein a pattern for determining the size and shape of the catalyst layer is formed into fine engraved shapes or fine embossed shapes on the surface of each of the pair of the metal drums and an insulating material is coated on the periphery of the pattern of each of the metal drums such that the voltage is applied only to the pattern for determining the size and shape of the catalyst layer when applying the voltage to the metal drums.

2. The method of claim 1 , further comprising drying the catalyst slurry applied to a surface of the metal drums by heating the metal drums.

3. The method of claim 1 , wherein the catalyst slurry is injected in a nitrogen atmosphere.

4. The method of claim 1 , further comprising: controlling a position and number of the sprays, a rotational speed of the drums, a distance between a surface of the sprays and a surface of each of the metal drums, and the voltage applied between the metal drums and the sprays according to an area of a catalyst layer formed on the surface of each of the metal drums and the amount of catalyst applied.

5. A method for manufacturing a fuel cell membrane-electrode assembly, the method comprising:
applying a voltage between one or more sprays spaced from a first metal drum and between one or more sprays spaced from a second metal drum;
spraying a catalyst slurry from each of the sprays toward the corresponding first and second metal drums, wherein the catalyst slurry and voltage cause a Coulomb explosion to coat the catalyst slurry on the metal drums as a catalyst layer; and
transferring the catalyst layer to both surfaces of a polymer electrolyte membrane fed between the metal drums,
wherein each of the metal drums comprises a pattern formed on a surface thereof to determine a size and a shape of a catalyst layer formed by the applied catalyst,
wherein the pattern is formed into fine engraved shapes or fine embossed shapes on the surface of each of the pair of the metal drums and an insulating material is coated on the periphery of the pattern of each of the metal drums such that the voltage is applied only to the pattern for determining the size and shape of the catalyst layer when applying the voltage to the metal drums.

6. The method of claim 5 , further comprising heating the metal drums to dry the catalyst slurry on the metal drums.

7. The method of claim 5 , wherein the catalyst slurry is sprayed in a nitrogen atmosphere.

8. The method of claim 5 , further comprising: controlling a position and number of the sprays, a rotational speed of the drums, a distance between a surface of the sprays and a surface of each of the metal drums, and the voltage applied between the metal drums and the sprays according to an area of a catalyst layer formed on the surface of each of the metal drums and the amount of catalyst applied.

9. The method of claim 5 , further comprising: feeding the polymer electrolyte membrane between the metal drums by rotation of the metal drums.

Assignees

• Lee Jae Seung
• Hyundai Motor Co Ltd

Inventors

• Lee Jae Seung

Classifications

• H01M4/8896

  Pressing, rolling, calendering (membrane electrode assemblies H01M8/1004) · CPC title

• B05C1/0813

  characterised by means for supplying liquid or other fluent material to the roller · CPC title

• H01M8/1004 Primary

  characterised by membrane-electrode assemblies [MEA] (H01M8/12 takes precedence) · CPC title

• H01M4/8853

  Electrodeposition · CPC title

• B05B5/08

  Plant for applying liquids or other fluent materials to objects · CPC title