Method for producing all solid-state battery, and all solid-state battery

Patent metadata

Field	Value
Publication number	US-2024250296-A1
Application number	US-202418584473-A
Country	US
Kind code	A1
Filing date	Feb 22, 2024
Priority date	Sep 21, 2018
Publication date	Jul 25, 2024
Grant date	—

Abstract

It is suppressed that an active material particle enters into or penetrates through a solid electrolyte layer when an active material layer and the solid electrolyte layer are pressed and that short circuits between a cathode and an anode occur. A method for producing an all solid-state battery includes: a first step of stacking an active material layer over at least one surface of a solid electrolyte layer to constitute a stack; and a second step of pressing the stack to constitute a compact, wherein in the first step, the active material layer contains a secondary particle of an active material, and in the second step, the secondary particle is crushed to primary particles by said pressing, the secondary particle being present in an interfacial portion between the active material layer and the solid electrolyte layer.

First claim

What is claimed is:

1 . A method for producing an all solid-state battery, the method comprising:
a first step of stacking a first active material layer over one surface of a solid electrolyte layer and a second active material layer over another surface of the solid electrolyte layer to constitute a stack, the first active material layer having an opposing part that is opposite to the second active material layer across the solid electrolyte layer, and an extending part that extends beyond the opposing part in a width direction, the first and second active material layers containing secondary particles of an active material, the stack having unevenness over surfaces of the first and second active material layers, the unevenness being caused by the secondary particles; and a second step of pressing the stack, and thereby, crushing, in the opposing part, the secondary particles to primary particles, the secondary particles being present in an interfacial portion between the first and second active material layers and the solid electrolyte layer, the primary particles having a diameter that is at most a one fifth of a diameter of the secondary particles, wherein after the second step, a proportion of a number of the secondary particles present in the interfacial portion within a range to which pressure is applied by the pressing is no more than 10% of a total number of the primary particles and the secondary particles, relation of 0<(X/Y)≤0.03 is satisfied wherein X is the diameter (μm) of the primary particle, and Y is a thickness (μm) of the solid electrolyte layer, the secondary particles present in the interfacial portion are crushed to the primary particles by the pressing to reduce the unevenness over the surfaces of the first and second active material layers in the interfacial portion, and after the pressing, a proportion of a number of the secondary particles in a total number of particles of the active material in the extending part is larger than a proportion of a number of the secondary particles in a total number of particles of the active material in the opposing part.

Assignees

• Toyota Motor Co Ltd

Inventors

• Isono Motoshi
• Ose Norihiro
• Suzuki Tomoya

Classifications

• H01M10/0585

  of accumulators having only flat construction elements, i.e. flat positive electrodes, flat negative electrodes and flat separators · CPC title

• H01M10/052 Primary

  Li-accumulators · CPC title

• H01M2300/0068

  inorganic · CPC title

• Y02P70/50

  Manufacturing or production processes characterised by the final manufactured product · CPC title

• Y02E60/10

  Energy storage using batteries · CPC title