Systems and methods for production of Xenon-133

Patent metadata

Field	Value
Publication number	US-12291448-B2
Application number	US-202318312989-A
Country	US
Kind code	B2
Filing date	May 5, 2023
Priority date	May 8, 2018
Publication date	May 6, 2025
Grant date	May 6, 2025

Abstract

Methods and systems for producing Xenon-133 are disclosed. A method for producing Xenon-133 includes collecting an off gas from a Molybdenum-99 production process in a storage tank. The off gas includes Xenon-133 and Krypton-85. The method further includes selectively adsorbing Xenon-133 from the off gas onto a charcoal column assembly such that Xenon-133 is selectively adsorbed onto the charcoal column assembly relative to Krypton-85. The method further includes desorbing the Xenon-133 from the charcoal column assembly by heating the charcoal column assembly, and condensing the Xenon-133 within a coil assembly.

First claim

What is claimed is:

1. A charcoal column assembly for separation of Xenon-133 from an off gas stream, the off gas stream generated during a Molybdenum-99 production process, the charcoal column assembly comprising:
a charcoal column having a volume of charcoal therein, the charcoal column having a top and a bottom;
a column flange having a first side and a second side, the column flange defining a flange inlet and a flange outlet, the charcoal column positioned on a first side of the column flange;
a fluid control assembly attached to the second side of the column flange, the fluid control assembly including an inlet assembly and an outlet assembly, wherein the top of the charcoal column is fluidly connected to the inlet assembly through the flange inlet; and
an outlet tube fluidly connected to the bottom of the charcoal column and to the outlet assembly through the flange outlet.

2. The charcoal column assembly of claim 1 , wherein the volume of charcoal includes a volume of activated charcoal.

3. The charcoal column assembly of claim 1 , wherein the volume of charcoal selectively adsorbs Xenon-133.

4. The charcoal column assembly of claim 1 , wherein the volume of charcoal selectively desorbs Xenon-133 when heated.

5. The charcoal column assembly of claim 1 , wherein the charcoal column defines a charcoal bed having a bed diameter in a range from about 20 mm to about 25 mm in length.

6. The charcoal column assembly of claim 1 , wherein the charcoal column assembly includes a mass of activated charcoal of between 15 grams and 45 grams.

7. A transportation vessel for transportation of Xenon-133, the transportation vessel comprising:
a charcoal column assembly comprising:
a charcoal column having a volume of charcoal therein, the charcoal column having a top and a bottom;
a column flange having a first side and a second side, the column flange defining a flange inlet and a flange outlet, the charcoal column positioned on a first side of the column flange;
a fluid control assembly attached to the second side of the column flange, the fluid control assembly including an inlet assembly and an outlet assembly, wherein the top of the charcoal column is fluidly connected to the inlet assembly through the flange inlet; and
an outlet tube fluidly connected to the bottom of the charcoal column and to the outlet assembly through the flange outlet;

a first nuclear radiation shield removably attached to the first side of the column flange, the first shield defining a first shield cavity, wherein the column assembly is positioned within the first shield cavity; and
a second nuclear radiation shield removably attached to the second side of the column flange, the second shield defining a second shield cavity, wherein the fluid control assembly is positioned within the second shield cavity;
wherein the first and second shields completely enclose the column assembly.

8. The transportation vessel of claim 7 , wherein the volume of charcoal includes a volume of activated charcoal.

9. The transportation vessel of claim 7 , wherein the volume of charcoal selectively adsorbs Xenon-133.

10. The transportation vessel of claim 7 , wherein the volume of charcoal selectively desorbs Xenon-133 when heated.

11. The transportation vessel of claim 7 , wherein the charcoal column defines a charcoal bed having a bed diameter in a range from about 20 mm to about 25 mm in length.

Assignees

• Curium Us Llc

Inventors

• Barbosa Luis Antonio M M
• Gerritsen Sven V
• Schackmann Martinus J A
• Gronland Paul A
• Hierholzer Brian

Classifications

• Y02C20/40

  of CO2 · CPC title

• F25J2215/36

  Xenon · CPC title

• F25J2270/904

  by liquid or gaseous cryogen in an open loop · CPC title

• F25J2205/20

  using solidification of components · CPC title

• F25J2210/42

  Nitrogen · CPC title