Method and system for forming and for catalytically reacting a reactant mixture—embodiment of the reactor

Patent metadata

Field	Value
Publication number	US-11065592-B2
Application number	US-201816759116-A
Country	US
Kind code	B2
Filing date	Oct 25, 2018
Priority date	Oct 25, 2017
Publication date	Jul 20, 2021
Grant date	Jul 20, 2021

Abstract

In a process as disclosed according to the present invention, gases or gas mixtures used to form a reactant mixture in an at least temporarily ignitable composition are fed into a mixing chamber ( 11 ) through the passages ( 131 ) in a boundary wall ( 13 ) of the mixing chamber ( 11 ) and by means of one or more feed conduits ( 14 ) which have feed orifices ( 141 ) and extend into the mixing chamber ( 11 ), respectively. The present invention likewise provides a corresponding reactor ( 1 ).

First claim

The invention claimed is:

1. Process for forming and for catalytically converting a gaseous reactant mixture in which a first gas or gas mixture and a second gas or gas mixture are mixed to give the reactant mixture and then supplied to a reaction zone ( 12 ) of a reactor ( 1 ), characterized in that the reactant mixture is at least temporarily formed as an ignitable gas mixture, and in that first gas or gas mixture and the second gas or gas mixture are fed into a mixing chamber ( 11 ) having a boundary wall ( 13 ) provided with a number of passages ( 131 ), where the first gas or gas mixture is fed into the mixing chamber ( 11 ) through the passages ( 131 ) in a critical flow state and the second gas or gas mixture is fed into the mixing chamber ( 11 ) by means of one or more feed conduits ( 14 ) which have feed orifices ( 141 ) and extend into the mixing chamber ( 11 ).

2. Process according to claim 1 , in which the first gas or gas mixture is provided on a side of the boundary wall ( 13 ) facing away from the mixing chamber ( 11 ) with a higher pressure than exists in the mixing chamber ( 11 ).

3. Process according to claim 1 , in which the second gas or gas mixture is fed into the mixing chamber ( 11 ) at a higher velocity than the laminar or turbulent flame velocity of the ignitable gas mixture and/or in a critical flow state.

4. Reactor ( 1 ) for formation and for catalytic conversion of a gaseous reactant mixture, wherein the reactor ( 1 ) has a reaction zone ( 12 ) and is set up to mix at least one first gas or gas mixture and one second gas or gas mixture to give the reactant mixture and supply it to the reaction zone ( 12 ), characterized in that the reactor ( 1 ) is set up to form the reactant mixture at least temporarily as an ignitable gas mixture, and in that the reactor ( 1 ) comprises a mixing chamber ( 11 ) having a boundary wall ( 13 ) provided with a number of passages ( 131 ), wherein the passages ( 131 ) are at least partially formed as nozzles having Venturi or Laval characteristics, wherein means set up to feed the first gas or gas mixture into the mixing chamber ( 11 ) through the passages ( 131 ) in a critical flow state are provided, and wherein one or more feed conduits ( 14 ) which have feed orifices ( 141 ) and extend into the mixing chamber ( 11 ) are provided for feeding of the second gas or gas mixture into the mixing chamber ( 11 ).

5. Process according to claim 1 , wherein the passages ( 131 ) are at least partly in the form of cylindrical holes.

6. Process according to claim 1 , wherein the passages ( 131 ) are at least partly in the form of nozzles.

7. Process according to claim 6 , wherein the passages ( 131 ) in the form of nozzles at least partly have Venturi or Laval characteristics.

8. Process according to claim 6 , wherein the passages ( 131 ) in the form of nozzles are at least partly exchangeable.

9. Process according to claim 1 , in which in the reactor ( 1 ) used the mixing chamber ( 11 ) has been provided with a random packing and/or a structured packing having a static mixing effect and/or with another mixing unit.

10. Process according to claim 1 , in which the one or more feed conduits ( 14 ) which has/have the feed orifices ( 141 ) and extend(s) into the mixing chamber ( 11 ) take(s) the form of tubular distributors.

11. Process according to claim 1 , in which in the reactor ( 1 ) used the mixing chamber ( 11 ) has a cylindrical interior, where a cross-sectional circular face of the cylindrical interior is formed by the boundary wall ( 13 ).

12. Process according to claim 11 , in which in the reactor ( 1 ) used the other cross-sectional circular face of the cylindrical interior is formed by a further boundary wall ( 15 ) having passages ( 151 ), where the further boundary wall ( 15 ) delimits the reaction zone ( 12 ) from the mixing chamber ( 11 ).

13. Process according to claim 12 , in which in the reactor ( 1 ) used the boundary walls ( 13 , 15 ) are secured to one another by means of stud bolts at a defined separation.

14. Process according to claim 1 , in which in the reactor ( 1 ) used the mixing chamber ( 11 ) is in explosion-resistant form.

15. Reactor according to claim 4 , wherein the passages ( 131 ) are at least partly in the form of cylindrical holes.

16. Reactor according to claim 4 , wherein the passages ( 131 ) are at least partly in the form of nozzles.

17. Reactor according to claim 16 , wherein the passages ( 131 ) in the form of nozzles at least partly have Venturi or Laval characteristics.

18. Reactor according to claim 16 , wherein the passages ( 131 ) in the form of nozzles are at least partly exchangeable.

Assignees

• Linde Ag

Inventors

• Wellenhofer Anton
• Zellhuber Mathieu
• Schubert Martin
• Birk Robert
• Pichler Celine
• Fritz Helmut

Classifications

• B01J2204/002

  the feeding side being of particular interest · CPC title

• B01J4/002

  Nozzle-type elements (nozzle-type reactors B01J19/26) · CPC title

• B01J19/305

  Supporting elements therefor, e.g. grids, perforated plates · CPC title

• B01J2208/00911

  Sparger-type feeding elements · CPC title

• B01J2219/2422

  Mixing means, e.g. fins or baffles attached to the monolith or placed in the channel · CPC title