Arrangement of electrochemical cells and the use of the same

Patent metadata

Field	Value
Publication number	US-10411274-B2
Application number	US-201615563153-A
Country	US
Kind code	B2
Filing date	Mar 23, 2016
Priority date	Mar 30, 2015
Publication date	Sep 10, 2019
Grant date	Sep 10, 2019

Abstract

The invention relates to an arrangement of electrochemical cells and also to the uses thereof. The electrochemical cells are arranged one above another and are in electrically conducting communication with one another. In this arrangement they form repeating units which in each case are formed of at least one interconnector, in which apertures for gas passage are formed, an electrochemical cell, which is formed of a cathode, an electrolyte and an anode, and contact elements on the anode side and on the cathode side, and are arranged one above another. The area of the individual planar electrochemical cells is in each case smaller than the area of the individual interconnectors, and the electrolytes finish flush in each case with a plane of a surface of the respective interconnector. Mounted on this surface of the interconnector in each case is a single sealing ply of a glass solder with constant thickness, for sealing the gap between electrolyte and interconnector (internal joining) and the gaps between apertures for gas passage of two adjacent interconnectors (external joining).

First claim

We claim:

1. An arrangement of electrochemical cells which are arranged one above another and in electrically conducting communication with one another, wherein said arrangement comprises a plurality of repeating units stacked upon each other, each repeating unit comprising at least one interconnector having opposing planar surfaces, said interconnector having apertures for gas passage, a planar electrochemical cell within said interconnector formed of a planar cathode, a planar anode, and an electrolyte between said cathode and anode, and further comprising cathode and anode contact elements, and
wherein the planar area of each electrochemical cell is smaller than the planar area of said interconnector, and
wherein the electrolyte is flush with one of said planar surfaces of the interconnector,
wherein each repeating unit further comprises a single planar sealing ply comprising a glass solder having constant thickness mounted upon each of said opposing planar surfaces of the interconnector for sealing any gaps between said electrolyte and the interconnector and sealing any gaps between said apertures for gas passage between two adjacent stacked interconnectors,
wherein said sealing ply is formed from plural glass solder sheet elements that are joined with each other at joins, wherein one sealing ply is mounted on one surface of said interconnector and another sealing ply is mounted on the opposing surface of the interconnector such that the joins of the sealing ply mounted on said one surface and the joins of the sealing ply mounted on said opposing surface are offset from each other in a direction perpendicular to the planes of the sealing plies.

2. The arrangement as claimed in claim 1 , wherein said arrangement is closed off with a top plate at one end side and with a baseplate on an opposite end side.

3. The arrangement as claimed in claim 1 , wherein said electrochemical cell is arranged inside of a recess which is formed in said interconnector.

4. The arrangement as claimed in claim 1 , wherein each said sealing ply has a maximum thickness deviation of 20%.

5. The arrangement as claimed in claim 1 , wherein said sealing plies on opposing surfaces of the interconnector have different thicknesses, the thickness of each individual sealing ply being constant.

6. The arrangement as claimed in claim 1 , wherein each sealing ply on opposing surfaces of said interconnector is arranged rotated by 180° from one another.

7. The arrangement as claimed in claim 1 , wherein said glass solder sheet elements are formed by robots for a fully automatic assembly.

8. The use of an arrangement as claimed in claim 1 as a fuel cell and/or electrolyzer.

Assignees

• Fraunhofer Ges Forschung

Inventors

• Megel Stefan
• Schadt Lutz
• Kusnezoff Mihails
• Schilm Jochen
• Trofimenko Nikolai

Classifications

• H01M8/0247

  characterised by the form (characterised by a channel configuration H01M8/0258) · CPC title

• C25B9/00

  Cells or assemblies of cells; Constructional parts of cells; Assemblies of constructional parts, e.g. electrode-diaphragm assemblies; Process-related cell features · CPC title

• H01M8/0276 Primary

  Sealing means characterised by their form (H01M8/0273 takes precedence) · CPC title

• H01M8/0258

  characterised by the configuration of channels, e.g. by the flow field of the reactant or coolant · CPC title

• H01M8/2425

  High-temperature cells with solid electrolytes · CPC title