Method of preparing nuclear fuel pellet including thermal conductive metal and nuclear fuel pellet prepared thereby

Patent metadata

Field	Value
Publication number	US-10102929-B2
Application number	US-201514591498-A
Country	US
Kind code	B2
Filing date	Jan 7, 2015
Priority date	May 26, 2014
Publication date	Oct 16, 2018
Grant date	Oct 16, 2018

Abstract

A method of a nuclear fuel pellet including a thermal conductive metal and a nuclear fuel pellet prepared thereby. The method includes preparing an oxide nuclear fuel granule having about 30%-45% theoretical density, mixing the fuel granule with thermal conductive metal powder, compacting the fuel granule with which the thermal conductive metal powder is mixed to prepare a green pellet, and sintering the green pellet. In the method, the sintering may be performed under a reducing gas atmosphere that is the same as the commercial pellet preparing process. Thus, compatibility compared to existing commercial preparing processes may be superior. Also, since a liquefied oxide formation process and a reducing process are omitted, the distribution uniformity of the metal material within the pellet may be superior. Therefore, the nuclear fuel pellet in which the metal network and fine microstructure are uniformly distributed within the pellet may be prepared.

First claim

What is claimed is:

1. A method of preparing a nuclear fuel pellet comprising a thermal conductive metal network, the method comprising:
preparing an oxide nuclear fuel granule having about 30% to about 45% theoretical density (T.D.);
mixing the prepared oxide nuclear fuel granule with a thermal conductive metal powder
compacting the oxide nuclear fuel granule with which the thermal conductive metal powder is mixed to prepare a green pellet; and
sintering the green pellet prepared.

2. The method as set forth in claim 1 , wherein the oxide nuclear fuel comprises at least one kind of metal oxide nuclear fuels selected from the consisting of UO 2 , PuO 2 , and ThO 2 .

3. The method as set forth in claim 1 , wherein the thermal conductive metal powder comprises at least one kind of metals selected from the group consisting of molybdenum (Mo), tungsten (W), and chromium (Cr).

4. The method as set forth in claim 1 , wherein the thermal conductive metal powder is mixed at a ratio of about 5 volume % to 15 volume % with respect to the oxide nuclear fuel granule.

5. The method as set forth in claim 1 , wherein the thermal conductive metal powder has a size of about 10 μm or less.

6. The method as set forth in claim 1 , wherein the green pellet is prepared at a compaction pressure of about 100 MPa to about 500 MPa.

7. The method as set forth in claim 1 , wherein the sintering is performed under a hydrogen gas atmosphere.

8. The method as set forth in claim 1 , wherein the sintering is performed at a temperature of about 1,300° C. to 1,800° C. for about 1 hour to about 10 hours.

9. The method as set forth in claim 1 , the nuclear fuel pellet comprises a thermal conductive metal having a network structure.

10. The method as set forth in claim 1 , wherein the nuclear fuel pellet has a density that is greater than about 96% theoretical density (T.D).

11. The method as set forth in claim 9 , wherein the thermal conductive metal having the network structure is distributed in at least one nuclear fuel pellet.

12. A method of improving thermal conductivity of a nuclear fuel pellet, the method comprising:
mixing an oxide nuclear fuel granule having about 30% to about 45% theoretical density (T.D.) with thermal conductive metal powder;
compacting the oxide nuclear fuel granule with which the thermal conductive metal powder is mixed to prepare a green pellet; and
sintering the green pellet,

wherein a network structure of a thermal conductive metal is formed in the pellet.

13. The method as set forth in claim 1 , wherein the prepared oxide nuclear fuel granule has a size of about 200 μm to about 1,000 μm.

14. The method as set forth in claim 12 , wherein the prepared oxide nuclear fuel granule has a size of about 200 μm to about 1,000 μm.

Assignees

• Korea Atomic Energy Res

Inventors

• Kim Dong-Joo
• Rhee Young Woo
• Kim Keon-Sik
• Kim Jong-Hun
• Oh Jangsoo
• Yang Jae-Ho
• Koo Yang-Hyun

Classifications

• Y02E30/38

  Cross-Sectional Technologies · mapped topic

• G21C2003/045

  Physics · mapped topic

• G21C3/04 Primary

  Constructional details · CPC title

• G21C21/02

  Manufacture of fuel elements or breeder elements contained in non-active casings · CPC title

• G21C3/623

  Oxide fuels · CPC title